On-Line HPLC as a Toolkit for Process Analytical Technology (PAT) in Pharmaceutical Processes

Process analytical technology (PAT) requiresvolume to control the collection of the product of
continuous monitoring of quality and this in turninterest as it elutes from the process
requires a model able to predict product qualitieschromatography column.
that can be measured in real-time from theThe issue with this approach is that it is totally
values of real-time process measurements.dependent on the reproducibility of the column
Process scale chromatography plays an importantelution profile which is impacted by column loading,
role in the purification of pharmaceutical products.purity of the starting material, column packing, and
Adjusting the eluent collection points allows thecolumn gradient generation.
process to compensate for the chromatography2. Collection of product based on column eluent
variability rather than increased variability in thevolume and optical density.
product purity. In addition to reducing productIn this approach, an in-line UV sensor set to 280
variability, using on-line HPLC also increasesnm is used to measure the absorbance from the
product yield, enables the use of increased levelsproduct’s peptide bonds. Since this is a non
of automation and reduces overall cycle time.product specific measurement, the OD
Determining where the product elution occurs,sensor’s output is examined in combination
generally involves collecting the column eluentwith the in-line flow meter to gain an additional
stream in small volumes that are sampled andlevel of resolution. That is, the product is only
analyzed in the laboratory utilizing higher resolutioncollected when the OD at 280 nm exceeds the
chromatographic techniques such asOD set point and falls within the volume set point
reversed-phase chromatography. This process ofwindow. This imparts greater selectivity than using
eluent fractionation and off-line chromatographicthe eluent volume approach alone, but is still
analysis is performed in process developmentdependent on the reproducibility of the
area in order to generate sufficient processcolumn’s elution profile.
understanding to enable when the product elutesAlthough the variability is less with this approach,
from the process scale chromatography column.the lack of a high level of selectivity still leads to
Fractionation of the column eluent has severalconservative collection set points that negatively
negative issues associated with it including:impact product yields.
- Degradation of product caused by the delays3. Measurement of product purity by on-line HPLC.
- Difficulty automating processing due to manualThe critical quality attribute of the product is its
handling of fractionspurity. Meeting a specified purity value is the
- Increased process cycle time caused by time tocriterion that determines if the process
obtain off-line assayschromatography step has been successful and if
- Labor intensivethe in-process material is suitable for forward
- Error may occurprocessing. By transferring the specificity of HPLC
- Reduced production capacity due to long cycleto an on-line analyzer, it is possible to directly
timesmeasure the critical quality attribute in near real
- Opportunities for product contaminationtime, thus allowing the process decision (i.e., when
- Storage required for “Work in Process”to start and stop collection of the product eluting
(the column fractions)from the process chromatography column) to be
Due to the many negative issues associated withbased on the critical quality attribute rather than
column fractionation, companies strive to eliminatebeing based on a surrogate measurement that is
this process operation as quickly as possible.impacted by the process variability.
Options to eliminate fractionation include:The increased emphasis on cost reduction and
1. Collection of product based on column eluentimproving production efficiency needs real-time
volume.process information. Product safety methodologies
In this approach, the eluent volume where theresult in an increased need to track product
product of sufficient purity is expected to elute isquality throughout the manufacturing process. So
determined from historical data and the startthis on-line HPLC helps to give advanced process
collection and stop collection set points are set. Ancontrol and real-time product release.
in-line flow meter is used to measure the eluent